Toward barrier free contact to molybdenum disulfide using graphene electrodes

Y Liu, H Wu, HC Cheng, S Yang, E Zhu, Q He… - Nano …, 2015 - ACS Publications
Nano letters, 2015ACS Publications
Two-dimensional layered semiconductors such as molybdenum disulfide (MoS2) have
attracted tremendous interest as a new class of electronic materials. However, there are
considerable challenges in making reliable contacts to these atomically thin materials. Here
we present a new strategy by using graphene as the back electrodes to achieve ohmic
contact to MoS2. With a finite density of states, the Fermi level of graphene can be readily
tuned by a gate potential to enable a nearly perfect band alignment with MoS2. We …
Two-dimensional layered semiconductors such as molybdenum disulfide (MoS2) have attracted tremendous interest as a new class of electronic materials. However, there are considerable challenges in making reliable contacts to these atomically thin materials. Here we present a new strategy by using graphene as the back electrodes to achieve ohmic contact to MoS2. With a finite density of states, the Fermi level of graphene can be readily tuned by a gate potential to enable a nearly perfect band alignment with MoS2. We demonstrate for the first time a transparent contact to MoS2 with zero contact barrier and linear output behavior at cryogenic temperatures (down to 1.9 K) for both monolayer and multilayer MoS2. Benefiting from the barrier-free transparent contacts, we show that a metal–insulator transition can be observed in a two-terminal MoS2 device, a phenomenon that could be easily masked by Schottky barriers found in conventional metal-contacted MoS2 devices. With further passivation by boron nitride (BN) encapsulation, we demonstrate a record-high extrinsic (two-terminal) field effect mobility up to 1300 cm2/(V s) in MoS2 at low temperature.
ACS Publications